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  1. Nanoscale industrial robots have potential as manufacturing platforms and are capable of automatically performing repetitive tasks to handle and produce nanomaterials with consistent precision and accuracy. We demonstrate a DNA industrial nanorobot that fabricates a three-dimensional (3D), optically active chiral structure from optically inactive parts. By making use of externally controlled temperature and ultraviolet (UV) light, our programmable robot, ~100 nanometers in size, grabs different parts, positions and aligns them so that they can be welded, releases the construct, and returns to its original configuration ready for its next operation. Our robot can also self-replicate its 3D structure and functions, surpassing single-step templating (restricted to two dimensions) by using folding to access the third dimension and more degrees of freedom. Our introduction of multiple-axis precise folding and positioning as a tool/technology for nanomanufacturing will open the door to more complex and useful nano- and microdevices.

     
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    Free, publicly-accessible full text available December 20, 2024
  2. Kamien, Randall ; Thomas, Jessica ; Chaté, Hugues ; Garisto, Robert ; Agarwal, Abhishek ; Dalena, Serena ; Mitra, Samindranath (Ed.)
    Sphere packing is an ancient problem. The densest packing is known to be a face-centered cubic (FCC) crystal, with space-filling fraction ϕFCC = pi/sqrt(18) ≈ 0.74. The densest “random packing,” random close packing (RCP), is yet ill defined, although many experiments and simulations agree on a value ϕRCP ≈ 0.64. We introduce a simple absorbing-state model, biased random organization (BRO), which exhibits a Manna class dynamical phase transition between absorbing and active states that has as its densest critical point ϕcmax ≈ 0.64 ≈ ϕRCP and, like other Manna class models, is hyperuniform at criticality. The configurations we obtain from BRO appear to be structurally identical to RCP configurations from other protocols. This leads us to conjecture that the highest-density absorbing state for an isotropic biased random organization model produces an ensemble of configurations that characterizes the state conventionally known as RCP. 
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  3. null (Ed.)
    Research on colloids is motivated by several factors. They can be used to answer fundamental questions related to the assembly of materials, and they have many potential applications in electronics, photonics, and life sciences. However, the rich variety of colloidal structures observed on the Earth can be influenced by the effects of gravity, which leads to particles settling and the motion of the surrounding fluid. To suppress the gravity effects, experiments on concentrated colloids of spherical and ellipsoidal fluorescent particles were carried out aboard the International Space Station. The particles were suspended in a decalin/tetralin mixture to match the particle refractive index. Confocal microscopy was used to visualize the particle behavior. The work was supported by the NSF CBET grants 1832260 and 1832291 and the NASA grant 80NSSC19K1655. 
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  4. null (Ed.)
    Research on colloids is motivated by several factors. They can be used to answer fundamental questions related to the assembly of materials, and they have many potential applications in electronics, photonics, and life sciences. However, the rich variety of colloidal structures observed on the Earth can be influenced by the effects of gravity, which leads to particles settling and the motion of the surrounding fluid. To suppress the gravity effects, experiments on concentrated colloids of spherical and ellipsoidal fluorescent particles were carried out aboard the International Space Station. The particles were suspended in a decalin/tetralin mixture to match the particle refractive index. Confocal microscopy was used to visualize the particle behavior. The work was supported by the NSF CBET grants 1832260 and 1832291 and the NASA grant 80NSSC19K1655. 
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  5. Abstract

    We introduce a hyperuniform-disordered platform for the realization of near-infrared photonic devices on a silicon-on-insulator platform, demonstrating the functionality of these structures in a flexible silicon photonics integrated circuit platform unconstrained by crystalline symmetries. The designs proposed advantageously leverage the large, complete, and isotropic photonic band gaps provided by hyperuniform disordered structures. An integrated design for a compact, sub-volt, sub-fJ/bit, hyperuniform-clad, electrically controlled resonant optical modulator suitable for fabrication in the silicon photonics ecosystem is presented along with simulation results. We also report results for passive device elements, including waveguides and resonators, which are seamlessly integrated with conventional silicon-on-insulator strip waveguides and vertical couplers. We show that the hyperuniform-disordered platform enables improved compactness, enhanced energy efficiency, and better temperature stability compared to the silicon photonics devices based on rib and strip waveguides.

     
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  6. Self-replication and exponential growth are ubiquitous in nature but until recently there were few examples of artificial self-replication. Often replication is a templated process where a parent produces a single offspring, doubling the population in each generation. Many species however produce more than one offspring at a time, enabling faster population growth and higher probability of species perpetuation. We have made a system of cross-shaped origami tiles that yields a number of offspring, four to eight or more, depending on the concentration of monomer units to be assembled. The parent dimer template serves as a seed to crystallize a one-dimensional crystal, a ladder. The ladder rungs are then UV–cross-linked and the offspring are then released by heating, to yield a litter of autonomous daughters. In the complement study, we also optimize the growth conditions to speed up the process and yield a 103increase in the growth rate for the single-offspring replication system. Self-replication and exponential growth of autonomous motifs is useful for fundamental studies of selection and evolution as well as for materials design, fabrication, and directed evolution. Methods that increase the growth rate, the primary evolutionary drive, not only speed up experiments but provide additional mechanisms for evolving materials toward desired functionalities.

     
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